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Spin fluctuations in the 112-type iron-based superconductor Ca 0.82 La 0.18 Fe 0.96 Ni 0.04 As 2 .

Tao XieChang LiuRyoichi KajimotoKazuhiko IkeuchiShiliang LiHuiqian Luo
Published in: Journal of physics. Condensed matter : an Institute of Physics journal (2022)
We report time-of-flight inelastic neutron scattering (INS) investigations on the spin fluctuation spectrum in the 112-type iron-based superconductor (FeSC) Ca 0.82 La 0.18 Fe 0.96 Ni 0.04 As 2 (CaLa-112). In comparison to the 122-type FeSCs with a centrosymmetric tetragonal lattice structure (space groupI4/mmm) at room temperature and an in-plane stripe-type antiferromagnetic (AF) order at low temperature, the 112 system has a noncentrosymmetric structure (space groupP21) with additional zigzag arsenic chains between Ca/La layers and a magnetic ground state with similar wavevectorQAFbut different orientations of ordered moments in the parent compounds. Our INS study clearly reveals that the in-plane dispersions and the bandwidth of spin excitations in the superconducting CaLa-112 closely resemble to those in 122 systems. While the total fluctuating moments⟨m2⟩≈4.6±0.2μB2/Fe are larger than 122 system, the dynamic correlation lengths are similar ( ξ  ≈ 10 Å). These results suggest that superconductivity in iron arsenides may have a common magnetic origin under similar magnetic exchange couplings with a dual nature from local moments and itinerant electrons, despite their different magnetic patterns and lattice symmetries.
Keyphrases
  • room temperature
  • molecularly imprinted
  • metal organic framework
  • ionic liquid
  • transition metal
  • single molecule
  • protein kinase
  • high resolution
  • liquid chromatography
  • monte carlo