Spectroscopy of phononic switching of magnetization in the terahertz gap.

All-optical schemes for switching magnetization offer a pathway towards the creation of more advanced data-storage technologies, both in terms of recording speed and energy-efficiency. It has previously been shown that picosecond-long optical pulses with central frequencies ranging between 12 and 30 THz are capable of driving magnetic switching in yttrium-iron-garnet films, provided that the excitation frequency matches the characteristic frequency of longitudinal optical phonons. Here, we explore how the phononic mechanism of magnetic switching in three distinct ferrimagnetic iron-garnet films evolves at optical frequencies below 10 THz, within the so-called terahertz gap. We find that at long wavelengths the magnetic switching rather correlates with phonon modes associated with the substrate. Our results show that the process of phononic switching of magnetization, previously discovered in the mid- to far-infrared spectral range, becomes much more complex at frequencies within the terahertz gap.