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Incarnatapeptins A and B, Nonribosomal Peptides Discovered Using Genome Mining and 1H/15N HSQC-TOCSY.

Kalindi D MorganDavid E WilliamsBrian O PatrickMarion RemigyCarmen A BanuelosMarianne D SadarKatherine S RyanRaymond J Andersen
Published in: Organic letters (2020)
Methods for the focused isolation of low-abundance natural products with specific chemical substructures could expand known bioactive chemical diversity for drug discovery. Here we report the combined use of genome mining and an 15N NMR-based screening method for the targeted isolation of the low-abundance piperazic-acid-containing peptides incarnatapeptins A (1) and B (3). Incarnatapeptin B (3) shows in vitro cytotoxicity to LNCaP prostate cancer cells.
Keyphrases
  • drug discovery
  • antibiotic resistance genes
  • magnetic resonance
  • genome wide
  • high resolution
  • amino acid
  • cancer therapy
  • dna methylation
  • gene expression
  • drug delivery
  • solid state
  • wastewater treatment