Scalable integrated two-dimensional Fourier-transform spectrometry.
Hongnan XuYue QinGaolei HuHon Ki TsangPublished in: Nature communications (2024)
Integrated spectrometers offer the advantages of small sizes and high portability, enabling new applications in industrial development and scientific research. Integrated Fourier-transform spectrometers (FTS) have the potential to realize a high signal-to-noise ratio but typically have a trade-off between the resolution and bandwidth. Here, we propose and demonstrate the concept of the two-dimensional FTS (2D-FTS) to circumvent the trade-off and improve scalability. The core idea is to utilize 2D Fourier transform instead of 1D Fourier transform to rebuild spectra. By combining a tunable FTS and a spatial heterodyne spectrometer, the interferogram becomes a 2D pattern with variations of heating power and arm lengths. All wavelengths are mapped to a cluster of spots in the 2D Fourier map beyond the free-spectral-range limit. At the Rayleigh criterion, the demonstrated resolution is 250 pm over a 200-nm bandwidth. The resolution can be enhanced to 125 pm using the computational method.
Keyphrases
- air pollution
- particulate matter
- heavy metals
- single molecule
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- polycyclic aromatic hydrocarbons
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- wastewater treatment
- optical coherence tomography
- magnetic resonance imaging
- water soluble
- density functional theory
- magnetic resonance
- human health
- high density
- mass spectrometry
- gas chromatography
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- contrast enhanced