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Nanomechanical Spectroscopy of 2D Materials.

Jan N KirchhofYuefeng YuGabriel AntheaumeGeorgy GordeevDenis YagodkinPeter ElliottDaniel B de AraújoSangeeta SharmaStephanie ReichKirill I Bolotin
Published in: Nano letters (2022)
We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a high Q silicon nitride nanomechanical resonator illuminated by a wavelength-tunable laser source. From the heating-related frequency shift of the resonator as well as its optical reflection measured as a function of photon energy, we obtain the real and imaginary parts of the dielectric function. Our measurements are unaffected by substrate-related screening and do not require any assumptions on the underling optical constants. This fast (τ rise ∼ 135 ns), sensitive (noise-equivalent power = 90 ⁣ pW √ Hz ), and broadband (1.2-3.1 eV, extendable to UV-THz) method provides an attractive alternative to spectroscopic or ellipsometric characterization techniques.
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