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Realizing highly efficient deep-blue organic light-emitting diodes towards Rec.2020 chromaticity by restricting the vibration of the molecular framework.

Chuan LiKai ZhangYanju LuoYang YangYong HuangMengjiao JiaYuling HeYue LeiJian-Xin TangYan HuangZhiyun Lu
Published in: Chemical science (2024)
Deep-blue organic light-emitting diodes (OLEDs) with narrow emission spectra and high efficiency, meeting the Rec.2020 standard, hold significant promise in the realm of 4K/8K ultrahigh-definition displays. However, the development of light-emitting materials exhibiting both narrowband emission and high efficiency, particularly in the realm of deep-blue thermally activated delayed fluorescence (TADF), confronts substantial challenges. Herein, a novel deep-blue TADF emitter, named BOC-PSi, was designed by integrating a rigid B-heterotriangulene acceptor (A) with a rigid phenazasiline donor (D). The replacement of a sp 3 carbon atom with a sp 3 silicon atom in the D moiety helps to restrict the low-frequency bending vibration throughout the entire D-A molecular backbone, while concurrently accelerating the multi-channel reverse intersystem crossing (RISC) processes. Notably, OLEDs using the BOC-PSi emitter exhibit exceptional performance, with a high maximum external quantum efficiency (EQE max ) approaching 20%, and a superior color purity closely aligning with the Rec.2020 blue standard.
Keyphrases
  • light emitting
  • high efficiency
  • highly efficient
  • molecular dynamics
  • single molecule
  • energy transfer
  • density functional theory
  • monte carlo