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High-Q Nanophotonics Over the Full Visible Spectrum Enabled by Hexagonal Boron Nitride Metasurfaces.

Lucca KühnerLuca SortinoBenjamin TilmannThomas WeberKenji WatanabeTakashi TaniguchiStefan A MaierAndreas Tittl
Published in: Advanced materials (Deerfield Beach, Fla.) (2022)
All-dielectric optical metasurfaces with high quality (Q) factors have so far been hampered by the lack of simultaneously lossless and high refractive index (RI) materials over the full visible spectrum. To achieve broad spectral coverage, the use of low-index materials is, in fact, unavoidable due to the inverse correlation between the band-gap energy (and therefore the optical losses) and the RI. However, for Mie resonant photonics, smaller RIs are associated with reduced Q factors and mode volume confinement. In this work, we leverage symmetry-broken quasi bound states in the continuum (qBICs) to efficiently suppress radiation losses from the low-index (n∼2) van der Waals material hexagonal boron nitride (hBN), realizing metasurfaces with high-Q resonances over the complete visible spectrum. In particular, we analyze the rational use of low and high RI materials as resonator components and harness our insights to experimentally demonstrate sharp qBIC resonances with Q factors above 300, spanning wavelengths between 400 nm and 1000 nm from a single hBN flake. Moreover, we utilize the enhanced electric near-fields to demonstrate second harmonic generation (SHG) with enhancement factors above 10 2 . Our results provide a theoretical and experimental framework for the implementation of low RI materials as photonic media for metaoptics. This article is protected by copyright. All rights reserved.
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