Fate of charge order in overdoped La-based cuprates.
Karin von ArxQisi WangS MustafiDaniel G MazzoneMasafumi HorioDeepak John MukkattukavilEkaterina PomjakushinaSunseng PyonT TakayamaHidenori TakagiT KurosawaN MomonoM OdaNicholas B BrookesD BettoWenliang ZhangTeguh Citra AsmaraYi TsengThorsten SchmittY SassaJohan ChangPublished in: npj quantum materials (2023)
In high-temperature cuprate superconductors, stripe order refers broadly to a coupled spin and charge modulation with a commensuration of eight and four lattice units, respectively. How this stripe order evolves across optimal doping remains a controversial question. Here we present a systematic resonant inelastic x-ray scattering study of weak charge correlations in La 2- x Sr x CuO 4 and La 1.8- x Eu 0.2 Sr x CuO 4 . Ultra high energy resolution experiments demonstrate the importance of the separation of inelastic and elastic scattering processes. Long-range temperature-dependent stripe order is only found below optimal doping. At higher doping, short-range temperature-independent correlations are present up to the highest doping measured. This transformation is distinct from and preempts the pseudogap critical doping. We argue that the doping and temperature-independent short-range correlations originate from unresolved electron-phonon coupling that broadly peaks at the stripe ordering vector. In La 2- x Sr x CuO 4 , long-range static stripe order vanishes around optimal doping and we discuss both quantum critical and crossover scenarios.