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Rhodium-Catalyzed Azine-Directed C-H Amidation with N -Methoxyamides.

Tao BanHuu-Manh VuJing ZhangJia-Yuan YongQiong LiuXu-Qin Li
Published in: The Journal of organic chemistry (2022)
Using N -methoxyamide reagents as an amide source, C-H amidation was realized at the ortho position of azine under the action of rhodium and boric acid. The method has mild reaction conditions, high atomic utilization, excellent yield, and wide adaptability to amidation reagents (both aromatic amides and fatty amides are applicable). Amide-substituted ketones can be obtained by a simple treatment and can be further transformed into bioactive substances. This provides a good supplement for the C-H bond amidation of aromatic rings.
Keyphrases
  • amino acid
  • molecular docking
  • room temperature
  • drinking water
  • molecular dynamics simulations
  • electron transfer