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Effective velocities of polaron spin states in monolayer transition metal dichalcogenides.

Yong SunXu-Fei MaXiao-Yi LiuYu CuiJia-Pei DengYao XiaoZhi-Qing LiZi-Wu Wang
Published in: Journal of physics. Condensed matter : an Institute of Physics journal (2021)
We propose a theoretical model for studying the effective velocities of polaron spin states in monolayer transition metal dichalcogenides (TMDS) on the substrate. It is found that the effective velocity of polaron shows the splitting with different magnitudes due to the Rashba spin-orbit coupling, which results in the reversed distribution of the effective velocities of polaron spin states. Moreover, the reversed points depend on the truncated wave-vector of optical phonon and can be modulated by the polarity of substrate and the internal distance between monolayer TMDS and substrate. These theoretical results enlighten some simple ways to distinguish and modulate the polaron spin states in two-dimensional heterostructures.
Keyphrases
  • transition metal
  • room temperature
  • density functional theory
  • high resolution
  • single molecule
  • structural basis