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Attosecond time-resolved photoelectron holography.

G PoratG AlonS RozenO PedatzurMichael KrügerD AzouryAdi NatanG OrensteinB D BrunerM J J VrakkingN Dudovich
Published in: Nature communications (2018)
Ultrafast strong-field physics provides insight into quantum phenomena that evolve on an attosecond time scale, the most fundamental of which is quantum tunneling. The tunneling process initiates a range of strong field phenomena such as high harmonic generation (HHG), laser-induced electron diffraction, double ionization and photoelectron holography-all evolving during a fraction of the optical cycle. Here we apply attosecond photoelectron holography as a method to resolve the temporal properties of the tunneling process. Adding a weak second harmonic (SH) field to a strong fundamental laser field enables us to reconstruct the ionization times of photoelectrons that play a role in the formation of a photoelectron hologram with attosecond precision. We decouple the contributions of the two arms of the hologram and resolve the subtle differences in their ionization times, separated by only a few tens of attoseconds.
Keyphrases
  • molecular dynamics
  • gas chromatography
  • high speed
  • high resolution
  • energy transfer
  • mass spectrometry
  • crystal structure
  • simultaneous determination
  • tandem mass spectrometry