Magnetic excitations in strained infinite-layer nickelate PrNiO 2 films.
Qiang GaoShiyu FanQisi WangJiarui LiXiaolin RenIzabela BiałoAnnabella DrewanowskiPascal RothenbühlerJaewon ChoiRonny SutartoYao WangTao XiangJiangping HuKe-Jin ZhouValentina BisogniRiccardo CominJohan ChangJonathan PelliciariXingjiang ZhouZhihai ZhuPublished in: Nature communications (2024)
Strongly correlated materials respond sensitively to external perturbations such as strain, pressure, and doping. In the recently discovered superconducting infinite-layer nickelates, the superconducting transition temperature can be enhanced via only ~ 1% compressive strain-tuning with the root of such enhancement still being elusive. Using resonant inelastic x-ray scattering (RIXS), we investigate the magnetic excitations in infinite-layer PrNiO 2 thin films grown on two different substrates, namely SrTiO 3 (STO) and (LaAlO 3 ) 0.3 (Sr 2 TaAlO 6 ) 0.7 (LSAT) enforcing different strain on the nickelates films. The magnon bandwidth of PrNiO 2 shows only marginal response to strain-tuning, in sharp contrast to the enhancement of the superconducting transition temperature T c in the doped superconducting samples. These results suggest the bandwidth of spin excitations of the parent compounds is similar under strain while T c in the doped ones is not, and thus provide important empirics for the understanding of superconductivity in infinite-layer nickelates.