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Quantum jamming transition to a correlated electron glass in 1T-TaS2.

Yaroslav A GerasimenkoIgor VaskivskyiMaksim LitskevichJan RavnikJaka VodebMichele DiegoViktor V KabanovDragan Mihailovic
Published in: Nature materials (2019)
Distinct many-body states may be created under non-equilibrium conditions through different ordering paths, even when their constituents are subjected to the same fundamental interactions. The phase-transition mechanism to such states remains poorly understood. Here, we show that controlled optical or electromagnetic perturbations can lead to an amorphous metastable state of strongly correlated electrons in a quasi-two-dimensional dichalcogenide. Scanning tunnelling microscopy reveals a hyperuniform pattern of localized charges, whereas multitip surface nanoscale conductivity measurements and tunnelling spectroscopy show an electronically gapless conducting state that is different from conventional Coulomb glasses and many-body localized systems. The state is stable up to room temperature and shows no signs of either local charge order or phase separation. The mechanism for its formation is attributed to a dynamical localization of electrons through mutual interactions. Theoretical calculations confirm the correlations between localized charges to be crucial for the state's unusual stability.
Keyphrases
  • room temperature
  • high resolution
  • molecular dynamics
  • single molecule
  • molecular dynamics simulations
  • ionic liquid
  • high speed
  • high frequency
  • monte carlo