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Anomalous phonon scattering and elastic correlations in amorphous solids.

Simon GelinHajime TanakaAnaël Lemaître
Published in: Nature materials (2016)
A major issue in materials science is why glasses present low-temperature thermal and vibrational properties that sharply differ from those of crystals. In particular, long-wavelength phonons are considerably more damped in glasses, yet it remains unclear how structural disorder at atomic scales affects such a macroscopic phenomenon. A plausible explanation is that phonons are scattered by local elastic heterogeneities that are essentially uncorrelated in space, a scenario known as Rayleigh scattering, which predicts that the damping of acoustic phonons scales with wavenumber k as kd+1 (in dimension d). Here we demonstrate that phonon damping scales instead as - kd+1 ln k, with this logarithmic enhancement originating from long-range spatial correlations of elastic disorder caused by similar stress correlations. Our work suggests that the presence of long-range spatial correlations of local stress and elasticity may well be the crucial feature that distinguishes amorphous solids from crystals.
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