Predictive Semiclassical Model for Coherent and Incoherent Emission in the Strong Field Regime: The Mollow Triplet Revisited.
Hsing-Ta ChenTao E LiAbraham NitzanJoseph E SubotnikPublished in: The journal of physical chemistry letters (2019)
We reinvestigate the famous Mollow triplet and show that most of the well-known quantum characteristics of the Mollow triplet-including incoherent emission and a nonstandard dependence of the sidebands on detuning-can be recovered quantitatively using semiclassical dynamics with a classical light field. In fact, by not relying on the rotating wave approximation, a semiclassical model predicts some quantum effects beyond the quantum optical Bloch equation, including higher-order scattering and asymmetric sideband features. This Letter highlights the fact that, with strong intensities, many putatively quantum features of light-matter interactions arise from a simple balance of mean-field electrodynamics and elementary spontaneous emission, which requires minimal computational cost. Our results suggest that the application of semiclassical electrodynamics to problems with strong light-matter coupling in the fields of nanophotonics and superradiance are likely to yield a plethora of new information.