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Magnetic Skyrmions above Room Temperature in a van der Waals Ferromagnet Fe 3 GaTe 2 .

Chen LiuSenfu ZhangHongyuan HaoHanin AlgaidiYinchang MaXingzhong Zhao
Published in: Advanced materials (Deerfield Beach, Fla.) (2024)
2D van der Waals (vdW) ferromagnetic crystals are a promising platform for innovative spintronic devices based on magnetic skyrmions, thanks to their high flexibility and atomic thickness stability. However, room-temperature skyrmion-hosting vdW materials are scarce, which poses a challenge for practical applications. In this study, a chemical vapor transport (CVT) approach is employed to synthesize Fe 3 GaTe 2 crystals and room-temperature Néel skyrmions are observed in Fe 3 GaTe 2 nanoflakes above 58 nm in thickness through in situ Lorentz transmission electron microscopy (L-TEM). Upon an optimized field cooling procedure, zero-field hexagonal skyrmion lattices are successfully generated in nanoflakes with an extended thickness range (30-180 nm). Significantly, these skyrmion lattices remain stable up to 355 K, setting a new record for the highest temperature at which skyrmions can be hosted. The research establishes Fe 3 GaTe 2 as an emerging above-room-temperature skyrmion-hosting vdW material, holding great promise for future spintronics.
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