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Nanoscale Noncollinear Spin Textures in Thin Films of a D2d Heusler Compound.

Ankit K SharmaJagannath JenaKumari Gaurav RanaAnastasios MarkouHolger L MeyerheimKatayoon MohseniAbhay K SrivastavaIlya KostanoskiyClaudia FelserStuart S P Parkin
Published in: Advanced materials (Deerfield Beach, Fla.) (2021)
Magnetic nano-objects, namely antiskyrmions and Bloch skyrmions, have been found to coexist in single-crystalline lamellae formed from bulk crystals of inverse tetragonal Heusler compounds with D2d symmetry. Here evidence is shown for magnetic nano-objects in epitaxial thin films of Mn2 RhSn formed by magnetron sputtering. These nano-objects exhibit a wide range of sizes with stability with respect to magnetic field and temperature that is similar to single-crystalline lamellae. However, the nano-objects do not form well-defined arrays, nor is any evidence found for helical spin textures. This is speculated to likely be a consequence of the poorer homogeneity of chemical ordering in the thin films. However, evidence is found for elliptically distorted nano-objects along perpendicular crystallographic directions within the epitaxial films, which is consistent with elliptical Bloch skyrmions observed in single-crystalline lamellae. Thus, these measurements provide strong evidence for the formation of noncollinear spin textures in thin films of Mn2 RhSn. Using these films, it is shown that individual nano-objects can be deleted using a local magnetic field from a magnetic tip and collections of nano-objects can be similarly written. These observations suggest a path toward the use of these objects in thin films with D2d symmetry as magnetic memory elements.
Keyphrases
  • room temperature
  • molecularly imprinted
  • ionic liquid
  • single molecule
  • transition metal
  • high resolution
  • atomic force microscopy
  • molecular dynamics