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Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators.

Elena Durán-ValdeiglesiasWeiwei ZhangCarlos Alonso-RamosSamuel SernaXavier Le RouxDelphine Maris-MoriniNiccolò CaselliFrancesco BiccariMassimo GurioliArianna FiloramoEric CassanLaurent Vivien
Published in: Scientific reports (2018)
Semiconducting single walled carbon nanotubes (s-SWNT) have an immense potential for the development of active optoelectronic functionalities in ultra-compact hybrid photonic circuits. Specifically, s-SWNT have been identified as a very promising solution to implement light sources in the silicon photonics platform. Still, two major challenges remain to fully exploit the potential of this hybrid technology: the limited interaction between s-SWNTs and Si waveguides and the low quantum efficiency of s-SWNTs emission. Silicon micro-ring resonators have the potential capability to overcome these limitations, by providing enhanced light s-SWNT interaction through resonant light recirculation. Here, we demonstrate that Si ring resonators provide SWNT chirality-wise photoluminescence resonance enhancement, releasing a new degree of freedom to tailor s-SWNT optical properties. Specifically, we show that judicious design of the micro-ring geometry allows selectively promoting the emission enhancement of either (8,6) or (8,7) SWNT chiralities present in a high-purity polymer-sorted s-SWNT solution. In addition, we present an analysis of nanometric-sized silicon-on-insulator waveguides that predicts stronger light s-SWNT interaction for transverse-magnetic (TM) modes than for conventionally used transverse-electric (TE) modes.
Keyphrases
  • carbon nanotubes
  • energy transfer
  • walled carbon nanotubes
  • human health
  • quantum dots
  • high throughput
  • solid state
  • molecular dynamics
  • molecularly imprinted
  • anaerobic digestion
  • ionic liquid
  • solid phase extraction