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Desymmetrization Process by Mg(II)-Catalyzed Intramolecular Vinylogous Michael Reaction.

Dan LiMinmin ZhangYuling YangTianyu PengDongxu YangWei GaoRui Wang
Published in: Organic letters (2020)
Chiral magnesium catalyzed intramolecular vinylogous Michael reaction of novel cyclohexadienones via a desymmetrization process is reported. (R)-BINOL derived ligand and an achiral amide were employed in the current in situ generated magnesium catalyst, giving the corresponding hydrogenated benzofuranone skeletons in good to excellent enantioselectivities with high yields. This simple and efficient strategy could be utilized for the synthesis of aromatized α,β-unsaturated ester and Br-substituted hydrogenated benzofuranone in good yields under mild conditions.
Keyphrases
  • room temperature
  • ionic liquid
  • energy transfer
  • molecular docking
  • electron transfer
  • metal organic framework
  • mass spectrometry