Nanoscopic jets and filaments of superfluid 4 He at zero temperature: A DFT study.
Francesco AncilottoManuel BarrancoMartí PiPublished in: The Journal of chemical physics (2023)
The instability of a cryogenic 4 He jet exiting through a small nozzle into vacuum leads to the formation of 4 He drops, which are considered ideal matrices for spectroscopic studies of embedded atoms and molecules. Here, we present a He-density functional theory (DFT) description of droplet formation resulting from jet breaking and contraction of superfluid 4 He filaments. Whereas the fragmentation of long jets closely follows the predictions of linear theory for inviscid fluids, leading to droplet trains interspersed with smaller satellite droplets, the contraction of filaments with an aspect ratio larger than a threshold value leads to the nucleation of vortex rings, which hinder their breakup into droplets.