Spin defects in hexagonal boron nitride for strain sensing on nanopillar arrays.
Tieshan YangNoah MendelsonChi LiAndreas GottschollJohn ScottMehran KianiniaVladimir DyakonovMilos TothIgor AharonovichPublished in: Nanoscale (2022)
Two-dimensional hexagonal boron nitride (hBN) has attracted much attention as a platform for studies of light-matter interactions at the nanoscale, especially in quantum nanophotonics. Recent efforts have focused on spin defects, specifically negatively charged boron vacancy (V B - ) centers. Here, we demonstrate a scalable method to enhance the V B - emission using an array of SiO 2 nanopillars. We achieve a 4-fold increase in photoluminescence (PL) intensity, and a corresponding 4-fold enhancement in optically detected magnetic resonance (ODMR) contrast. Furthermore, the V B - ensembles provide useful information about the strain fields associated with the strained hBN at the nanopillar sites. Our results provide an accessible way to increase the emission intensity as well as the ODMR contrast of the V B - defects, while simultaneously form a basis for miniaturized quantum sensors in layered heterostructures.
Keyphrases
- magnetic resonance
- quantum dots
- room temperature
- molecular dynamics
- density functional theory
- contrast enhanced
- high intensity
- energy transfer
- reduced graphene oxide
- high throughput
- transition metal
- single molecule
- working memory
- high density
- quality improvement
- atomic force microscopy
- magnetic resonance imaging
- gold nanoparticles
- monte carlo