High-order harmonic generation by static coherent states method in single-electron atomic and molecular systems.

We solve the time-dependent Schrodinger equation using the coherent states as basis sets for computing high harmonic generation (HHG) in a full-dimensional single-electron "realistic" system. We apply the static coherent states (SCS) method to investigate HHG in the hydrogen molecular ion induced by a linearly polarized laser field. We show that SCS gives reasonable agreement compared to the three dimensional unitary split-operator approach. Next, we study isolated attosecond pulse generation in H 2 + . To do so, we employ the well-known polarization gating technique, which combines two delayed counter-rotating circular laser pulses, and opens up a gate at the central portion of the superposed pulse. Our results suggest that the SCS method can be used for full-dimensional quantum simulation of higher dimensional systems such as the hydrogen molecule in the presence of an external laser field.