Engineering lithiophilic Ni-Al@LDH interlayers on a garnet-type electrolyte for solid-state lithium metal batteries.
Wei LiuGuanjie LuZuguang YangQiannan ZhaoXiaolin HuDan WuZongyang LiRonghua WangShikuan SunChaohe XuPublished in: Chemical communications (Cambridge, England) (2021)
In this work, a lithiophilic Ni-Al@LDH interlayer is engineered at the Li6.4La3Zr1.4Ta0.6O12 (LLZTO) electrolyte and Li anode interface. The Ni-Al@LDH interlayer can significantly reduce the interfacial resistance as well as give excellent cycling performance both in a symmetric Li//Li cell and solid full lithium metal batteries.