Optical Microfluidic Waveguides and Solution Lasers of Colloidal Semiconductor Quantum Wells.
Joudi MaskounNegar GheshlaghiFurkan IsikSavas DelikanliOnur ErdemEmine Yegan ErdemHilmi Volkan DemirPublished in: Advanced materials (Deerfield Beach, Fla.) (2021)
The realization of high-quality lasers in microfluidic devices is crucial for numerous applications, including biological and chemical sensors and flow cytometry, and the development of advanced lab-on-chip (LOC) devices. Herein, an ultralow-threshold microfluidic single-mode laser is proposed and demonstrated using an on-chip cavity. CdSe/CdS@Cdx Zn1- x S core/crown@gradient-alloyed shell colloidal semiconductor quantum wells (CQWs) dispersed in toluene are employed in the cavity created inside a poly(dimethylsiloxane) (PDMS) microfluidic device using SiO2 -protected Ag mirrors to achieve in-solution lasing. Lasing from such a microfluidic device having CQWs solution as a microfluidic gain medium is shown for the first time with a record-low optical gain threshold of 17.1 µJ cm- ² and lasing threshold of 68.4 µJ cm- ² among all solution-based lasing demonstrations. In addition, air-stable SiO2 protected Ag films are used and designed to form highly tunable and reflective mirrors required to attain a high-quality Fabry-Pérot cavity. These realized record-low thresholds emanate from the high-quality on-chip cavity together with the core/crown@gradient-alloyed shell CQWs having giant gain cross-section and slow Auger rates. This microfabricated CQW laser provides a compact and inexpensive coherent light source for microfluidics and integrated optics covering the visible spectral region.
Keyphrases
- circulating tumor cells
- high throughput
- single cell
- quantum dots
- flow cytometry
- high speed
- room temperature
- label free
- high resolution
- molecular dynamics
- magnetic resonance imaging
- heavy metals
- heart failure
- computed tomography
- energy transfer
- solid state
- risk assessment
- low cost
- left ventricular
- mass spectrometry
- highly efficient
- light emitting