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Measurement of the magnetic octupole susceptibility of PrV 2 Al 20 .

Linda YeMatthew E SorensenMaja D BachmannIan R Fisher
Published in: Nature communications (2024)
Revealing the presence of magnetic octupole order and associated octupole fluctuations in solids is a highly challenging task due to the lack of simple external fields that can couple to magnetic octupoles. Here, we demonstrate a methodology for probing the magnetic octupole susceptibility of a candidate material, PrV 2 Al 20 , using a product of magnetic field H i and shear strain ϵ jk as a composite effective field, while employing an adiabatic elastocaloric effect to probe the response. We observe Curie-Weiss behavior in the obtained octupolar susceptibility down to approximately 3 K. Although octupole order does not appear to be the leading multipolar channel in PrV 2 Al 20 , our results nevertheless reveal the presence of strong magnetic octupole fluctuations and hence demonstrate that octupole order is at least a competing state. More broadly, our results highlight how anisotropic strain can be combined with magnetic fields to probe elusive 'hidden' electronic orders.
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