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Large-bias spectroscopy of Yu-Shiba-Rusinov states in a double quantum dot.

Heidi PottsMarkus AspegrenRousan DebbarmaSebastian LehmannClaes Thelander
Published in: Nanotechnology (2023)
We have performed tunnel transport spectroscopy on a quantum dot (QD) molecule proximitized by a superconducting contact. In such a system, the scattering between QD spins and Bogoliubov quasiparticles leads to the formation of Yu-Shiba-Rusinov (YSR) states within the superconducting gap. In this work, we investigate interactions appearing when one- and two-electron spin states in a double-QD energetically align with the superconducting gap edge. We find that the inter-dot spin-triplet state interacts considerably stronger with the superconductor than the corresponding singlet, pointing to stronger screening. By forming a ring molecule with a significant orbital contribution to the effective g -factor, we observe interactions of all four spin-orbital one-electron states with the superconductor under a weak magnetic field.
Keyphrases
  • single molecule
  • room temperature
  • density functional theory
  • high resolution
  • energy transfer
  • transition metal
  • mass spectrometry
  • electron transfer
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