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Palladium-Catalyzed Chemoselective and Biocompatible Functionalization of Cysteine-Containing Molecules at Room Temperature.

Riyadh Ahmed Atto Al-ShuaeebSergii KolodychOleksandr KonievSébastien DelacroixStéphane ErbStéphanie NicolaÿJean-Christophe CintratJean-Daniel BrionSarah CianféraniMouâd AlamiAlain WagnerSamir Messaoudi
Published in: Chemistry (Weinheim an der Bergstrasse, Germany) (2016)
The third generation of aminobiphenyl palladacycle pre-catalyst "G3-Xantphos" enables functionalization of peptides containing cysteine in high yields. The conjugation (bioconjugation) occurs chemoselectively at room temperature under biocompatible conditions. Extension of the method to protein functionalization allows selective bioconjugation of the trastuzumab antibody.
Keyphrases
  • room temperature
  • ionic liquid
  • fluorescent probe
  • drug release
  • amino acid
  • epidermal growth factor receptor
  • protein protein
  • drug delivery
  • single molecule
  • highly efficient