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A Highly Asymmetric Gold(III) η3 -Allyl Complex.

Marte Sofie Martinsen HolmsenAinara NovaSigurd Øien-ØdegaardRichard H HeynMats Tilset
Published in: Angewandte Chemie (International ed. in English) (2019)
A highly asymmetric AuIII η3 -allyl complex has been generated by treating Au(η1 -allyl)Br(tpy) (tpy=2-(p-tolyl)pyridine) with AgNTf2 . The resulting η3 -allyl complex has been characterized by NMR spectroscopy and X-ray crystallography. DFT calculations and variable temperature 1 H NMR suggest that the allyl ligand is highly fluxional.
Keyphrases
  • high resolution
  • density functional theory
  • solid state
  • magnetic resonance
  • molecular dynamics
  • magnetic resonance imaging
  • gold nanoparticles
  • visible light