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Fast electrodeposition of zinc onto single zinc nanoparticles.

Giorgia ZampardiRichard G Compton
Published in: Journal of solid state electrochemistry : current research and development in science and technology (2020)
The zinc deposition reaction onto metallic zinc has been investigated at the single particle level through the electrode-particle collision method in neutral solutions, and in respect of its dependence on the applied potential and the ionic strength of a sulphate-containing solution. Depending on the concentration of sulphate ions in solution, different amounts of metallic zinc were deposited on the single Zn nanoparticles. Specifically, insights into the electron transfer kinetics at the single particles were obtained, indicating an electrically early reactant-like transition state, which is consistent with the rate-determining partial de-hydration/de-complexation process. Such information on the reaction kinetics at the nanoscale is of vital importance for the development of more efficient and long-lasting nanostructured Zn-based negative electrodes for Zn-ion battery applications.
Keyphrases
  • oxide nanoparticles
  • electron transfer
  • solid state
  • heavy metals
  • high resolution
  • quantum dots
  • gold nanoparticles
  • aqueous solution
  • climate change
  • walled carbon nanotubes