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Fast electrical modulation of strong near-field interactions between erbium emitters and graphene.

Daniel CanoAlban FerrierKaruppasamy SoundarapandianAntoine Reserbat-PlanteyMarion ScarafagioAlexandre TallaireAntoine SeyeuxPhilippe MarcusHugues de RiedmattenPhilippe GoldnerFrank H L KoppensKlaas-Jan Tielrooij
Published in: Nature communications (2020)
Combining the quantum optical properties of single-photon emitters with the strong near-field interactions available in nanophotonic and plasmonic systems is a powerful way of creating quantum manipulation and metrological functionalities. The ability to actively and dynamically modulate emitter-environment interactions is of particular interest in this regard. While thermal, mechanical and optical modulation have been demonstrated, electrical modulation has remained an outstanding challenge. Here we realize fast, all-electrical modulation of the near-field interactions between a nanolayer of erbium emitters and graphene, by in-situ tuning the Fermi energy of graphene. We demonstrate strong interactions with a  >1000-fold increased decay rate for  ~25% of the emitters, and electrically modulate these interactions with frequencies up to 300 kHz - orders of magnitude faster than the emitter's radiative decay (~100 Hz). This constitutes an enabling platform for integrated quantum technologies, opening routes to quantum entanglement generation by collective plasmon emission or photon emission with controlled waveform.
Keyphrases
  • light emitting
  • molecular dynamics
  • energy transfer
  • monte carlo
  • room temperature
  • high resolution
  • walled carbon nanotubes
  • quantum dots
  • living cells