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A Terminal Chlorophosphinidene Complex.

Josh AbbensethSven Schneider
Published in: Zeitschrift fur anorganische und allgemeine Chemie (2020)
Terminal, electrophilic phosphinidene complexes (M=PR) are attractive platforms for PR-transfer to organic substrates. In contrast to aryl- or alkylphosphinidene complexes terminal chlorophosphinidenes (M=PCl) have only been proposed as transient intermediates but isolable example remain elusive. Here we present the transfer of PCl from chloro-substituted dibenzo-7λ3-phosphanorbornadiene to a square-planar osmium(II) PNP pincer complex to give the first isolable, terminal chlorophosphinidene complex with remarkable thermal stability. Os=P bonding was examined computationally giving rise to highly covalent {OsII=PICl} double bonding.
Keyphrases
  • molecular docking
  • magnetic resonance imaging
  • computed tomography
  • blood brain barrier