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Controlling the Polarization of Nitrogen Ion Lasing.

Jingsong GaoXiang ZhangYang WangJiahao DongMingwei LeiYi LiuChengyin WuQihuang GongHongbing Jiang
Published in: The journal of physical chemistry letters (2024)
Air lasing provides a promising technique to remotely produce coherent radiation in the atmosphere and has attracted continuous attention. However, the polarization properties of N 2 + lasing with seeding have not been understood since it was discovered 10 years ago, in which the polarization behaviors appear disordered and confusing. Here, we performed an experimental and theoretical investigation of the polarization properties of N 2 + lasing and successfully revealed its underlying physical mechanism. We found that the optical gain is anisotropic, owing to the permanent alignment of N 2 + induced by the preferential ionization of the pump light. As a result, the polarization of the N 2 + lasing tends to align with that of the pump light after amplification, which becomes more pronounced as the amplification factor increases. Based on the permanent alignment of N 2 + , we built a theoretical model that analytically interpreted and numerically reproduced the experimental observations, which points out the key factors for controlling the polarization of N 2 + lasing.
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