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Topotactic fabrication of transition metal dichalcogenide superconducting nanocircuits.

Xiaohan WangHao WangLiang MaLabao ZhangZhuolin YangDaxing DongXi ChenHaochen LiYanqiu GuanBiao ZhangQi ChenLili ShiHui LiZhi QinXuecou TuLijian ZhangXiao-Qing JiaJian ChenLin KangPeiheng Wu
Published in: Nature communications (2023)
Superconducting nanocircuits, which are usually fabricated from superconductor films, are the core of superconducting electronic devices. While emerging transition-metal dichalcogenide superconductors (TMDSCs) with exotic properties show promise for exploiting new superconducting mechanisms and applications, their environmental instability leads to a substantial challenge for the nondestructive preparation of TMDSC nanocircuits. Here, we report a universal strategy to fabricate TMDSC nanopatterns via a topotactic conversion method using prepatterned metals as precursors. Typically, robust NbSe 2 meandering nanowires can be controllably manufactured on a wafer scale, by which a superconducting nanowire circuit is principally demonstrated toward potential single photon detection. Moreover, versatile superconducting nanocircuits, e.g., periodical circle/triangle hole arrays and spiral nanowires, can be prepared with selected TMD materials (NbS 2 , TiSe 2 , or MoTe 2 ). This work provides a generic approach for fabricating nondestructive TMDSC nanocircuits with precise control, which paves the way for the application of TMDSCs in future electronics.
Keyphrases
  • transition metal
  • room temperature
  • human health
  • risk assessment
  • climate change
  • high density
  • life cycle