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s -Tetrazine-Bridged Photochromic Aromatic Framework Material.

Tao ChenGuangjun XiaoZhuo WangJian ZouJian WangWei-Bo HuYahu A LiuHui YangKe Wen
Published in: ACS omega (2022)
Integrating fluorescent chromophores in aromatic frameworks could not only prevent aggregation-induced quenching caused by the π-π stacking interaction between the chromophore components but also confer new fluorescence properties. Herein, we report the fabrication of s -tetrazine-bridged aromatic frameworks TzAF by the incorporation of the smallest aromatic fluorophore, s -tetrazine ( Tz ), into the skeleton of a tetrahedrally connected lattice of aromatic frameworks. The thin films of TzAF coated on silica gel plates were found to exhibit reversible photoswitching fluorescence characteristics under alternate UV and visible-light irradiations with excellent fluorescence stability and high on/off contrast. The repeatable "on/off"fluorescence photoswitchability of the TzAF thin films was mechanistically attributed to light-induced reversible transformation between TzAF 's neutral and radical states.
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