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Electrospinning-assisted porous skeleton electrolytes for semi-solid Li-O 2 batteries.

Jing WuMinghui LiShasha GaoYaying DouKecheng PanZhang ZhangZhang Zhang
Published in: Chemical communications (Cambridge, England) (2024)
Solid-state lithium-oxygen batteries offer great promise in meeting the practical demand for high-energy-density and safe energy storage. We have developed fibrous gel polymer electrolytes (GPEs) using a polyacrylonitrile (PAN) matrix via electrospinning. The 3D structure of GPEs enhances electrolyte absorption, while the interconnected design promotes strong interactions between Li + and polar groups within the PAN matrix, thereby improving ion transport efficiency. In practical tests, both lithium symmetric cells and Li-O 2 batteries demonstrated the ability to operate at high current densities over long cycles.
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