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Ru(II)-Catalyzed C-H Hydroxyalkylation and Mitsunobu Cyclization of N-Aryl Phthalazinones.

Kunyoung KimSang Hoon HanDaeun JeoungPrithwish GhoshSaegun KimSeung Jun KimJin-Mo KuNeeraj Kumar MishraIn Su Kim
Published in: The Journal of organic chemistry (2020)
Ruthenium(II)-catalyzed C(sp2)-H functionalization of N-aryl phthalazinones with a range of aldehydes and activated ketone is described. Initial formation of hydroxyalkylated phthalazinones and subsequent Mitsunobu cyclization provided facile access to biologically relevant indazolophthalazinones. The utility of this method is highlighted by synthetic transformations into a series of potentially bioactive scaffolds.
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