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A mixed-spin spin-crossover thiozolylimine [Fe4L6]8+ cage.

Li LiAlexander R CrazeOuti MustonenHikaru ZennoJacob J WhittakerShinya HayamiLeonard F LindoyChristopher E MarjoJack Kay CleggJanice Rae Aldrich-WrightFeng Li
Published in: Dalton transactions (Cambridge, England : 2003) (2019)
The self-assembly of a mixed-spin [Fe4L6]8+ tetrahedral cage is reported. The cage undergoes temperature induced spin-crossover with a 29 K hystereisis. Variable temperature X-ray photoelectron spectroscopy (VT-XPS), combined with SQUID data, allowed differentiation between the surface and bulk magnetic properties.
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