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Strongly Cavity-Enhanced Spontaneous Emission from Silicon-Vacancy Centers in Diamond.

Jingyuan Linda ZhangShuo SunMichael J BurekConstantin DoryYan-Kai TzengKevin A FischerYousif KelaitaKonstantinos G LagoudakisMarina RadulaskiZhi-Xun ShenNicholas A MeloshSteven ChuMarko LončarJelena Vučković
Published in: Nano letters (2018)
Quantum emitters are an integral component for a broad range of quantum technologies, including quantum communication, quantum repeaters, and linear optical quantum computation. Solid-state color centers are promising candidates for scalable quantum optics due to their long coherence time and small inhomogeneous broadening. However, once excited, color centers often decay through phonon-assisted processes, limiting the efficiency of single-photon generation and photon-mediated entanglement generation. Herein, we demonstrate strong enhancement of spontaneous emission rate of a single silicon-vacancy center in diamond embedded within a monolithic optical cavity, reaching a regime in which the excited-state lifetime is dominated by spontaneous emission into the cavity mode. We observe 10-fold lifetime reduction and 42-fold enhancement in emission intensity when the cavity is tuned into resonance with the optical transition of a single silicon-vacancy center, corresponding to 90% of the excited-state energy decay occurring through spontaneous emission into the cavity mode. We also demonstrate the largest coupling strength (g/2π = 4.9 ± 0.3 GHz) and cooperativity (C = 1.4) to date for color-center-based cavity quantum electrodynamics systems, bringing the system closer to the strong coupling regime.
Keyphrases
  • energy transfer
  • molecular dynamics
  • solid state
  • monte carlo
  • high resolution
  • high speed
  • quantum dots
  • high intensity
  • ionic liquid
  • molecularly imprinted
  • solid phase extraction