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Stable continuous-wave lasing from discrete cesium lead bromide quantum dots embedded in a microcavity.

Hongbo ZhangWen WenBowen DuLei ZhouYu ChenShun FengChenji ZouLishu WuHong Jin FanWeibo GaoHandong SunJingzhi ShangTing Yu
Published in: Nanoscale horizons (2023)
All-inorganic cesium lead bromide (CsPbBr 3 ) quantum dots (QDs) with high photoluminescence (PL) quantum efficiency have been reported as ideal gain materials for high-performance lasers. Nevertheless, isolated CsPbBr 3 QDs have not achieved lasing emission (LE) due to finite absorption cross-section. Here, we demonstrate continuous-wave lasing of isolated CsPbBr 3 QDs embedded in a microcavity. Distributed Bragg reflectors (DBRs), together with isolated CsPbBr 3 QDs in a polymer matrix, are introduced to construct a vertical-cavity surface-emitting laser (VCSEL), which exhibits stable single-mode lasing emissions with an ultra-low threshold of 8.8 W cm -2 and a high Q factor of 1787. Such perovskite-based microcavity structures sustain highly stable excitons at room temperature and can provide an excellent experimental platform to further study the single-particle nano-lasers and quantum physics frontiers such as exciton-polariton condensation, single-photon emission, and optical quantum communication.
Keyphrases
  • quantum dots
  • energy transfer
  • room temperature
  • high resolution
  • molecular dynamics
  • sensitive detection
  • ionic liquid
  • high speed
  • high throughput
  • high efficiency
  • single cell
  • solar cells
  • water soluble