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Attosecond field emission.

H Y KimManish GargS MandalLennart SeiffertThomas FennelE Goulielmakis
Published in: Nature (2023)
Field emission of electrons underlies great advances in science and technology, ranging from signal processing at ever higher frequencies 1 to imaging of the atomic-scale structure of matter 2 with picometre resolution. The advancing of electron microscopy techniques to enable the complete visualization of matter on the native spatial (picometre) and temporal (attosecond) scales of electron dynamics calls for techniques that can confine and examine the field emission on sub-femtosecond time intervals. Intense laser pulses have paved the way to this end 3,4 by demonstrating femtosecond confinement 5,6 and sub-optical cycle control 7,8 of the optical field emission 9 from nanostructured metals. Yet the measurement of attosecond electron pulses has remained elusive. We used intense, sub-cycle light transients to induce optical field emission of electron pulses from tungsten nanotips and a weak replica of the same transient to directly investigate the emission dynamics in real time. Access to the temporal properties of the electron pulses rescattering off the tip surface, including the duration τ = (53 as ± 5 as) and chirp, and the direct exploration of nanoscale near fields open new prospects for research and applications at the interface of attosecond physics and nano-optics.
Keyphrases
  • electron microscopy
  • high resolution
  • high speed
  • solid state
  • molecular dynamics
  • minimally invasive
  • risk assessment
  • mass spectrometry
  • electron transfer
  • climate change