Normal-Incidence-Excited Strong Coupling between Excitons and Symmetry-Protected Quasi-Bound States in the Continuum in Silicon Nitride-WS2 Heterostructures at Room Temperature.
Shun CaoHongguang DongJinlong HeErik ForsbergYi JinSailing HePublished in: The journal of physical chemistry letters (2020)
Room-temperature strong coupling between quasi-bound states in the continuum (q-BIC) of a silicon nitride metasurface and excitons in a WS2 monolayer is investigated in detail by both numerical simulations and theoretical calculations. The strong coupling between the q-BIC mode and excitons leads to a remarkable spectral splitting and typical anticrossing behavior of the Rabi splitting, which can be realized in the absorption spectra by varying the grating thickness and asymmetry parameter of the silicon-nitride metasurface, respectively. In addition, both the line width of the q-BIC mode and local electric field enhancement are found to affect the strong coupling, which needs to be considered in detail in q-BIC metasurface designs. This work provides a possible way to enhance light-matter interactions in transition metal dichalcogenides monolayers and pave the way for future quantum and nanophotonic applications.
Keyphrases
- room temperature
- ionic liquid
- molecular dynamics
- quantum dots
- transition metal
- optical coherence tomography
- density functional theory
- monte carlo
- reduced graphene oxide
- magnetic resonance imaging
- energy transfer
- computed tomography
- magnetic resonance
- molecular dynamics simulations
- solid state
- mass spectrometry
- single molecule
- electron transfer