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Hybrid Moiré Excitons and Trions in Twisted MoTe 2 -MoSe 2 Heterobilayers.

Shen ZhaoXin HuangRoland GillenZhijie LiSong LiuKenji WatanabeTakashi TaniguchiJanina MaultzschJames C HoneAlexander HögeleAnvar S Baimuratov
Published in: Nano letters (2024)
We report experimental and theoretical studies of MoTe 2 -MoSe 2 heterobilayers with rigid moiré superlattices controlled by the twist angle. Using an effective continuum model that combines resonant interlayer electron tunneling with stacking-dependent moiré potentials, we identify the nature of moiré excitons and the dependence of their energies, oscillator strengths, and Landé g -factors on the twist angle. Within the same framework, we interpret distinct signatures of bound complexes among electrons and moiré excitons in nearly collinear heterostacks. Our work provides a fundamental understanding of hybrid moiré excitons and trions in MoTe 2 -MoSe 2 heterobilayers and establishes the material system as a prime candidate for optical studies of correlated phenomena in moiré lattices.
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