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Nitrogen and magnesium codoped biochar activates periodate to remediate bensulfuron methyl-contaminated water at low temperature: Performance, mechanisms, and phytotoxicity.

Yang YangZhichao KangGuanghui XuYong Yu
Published in: Journal of hazardous materials (2024)
Bensulfuron methyl (BSM), a typical sulfonylurea herbicide, has been widely used worldwide for weed suppression and crop protection. Nevertheless, the long-term and prolonged usage led to residues in environment, resulting in the reduction of crop yields and even threatening food security. In this study, the nitrogen/magnesium codoped biochar (NMg-BC) was prepared via two-step pyrolysis method to activate periodate (PI) for BSM degradation. The results demonstrated BSM degradation rate was 87.9 % within 10 min by NMg-BC/PI system at 15 ℃. The system exhibited the favorable tolerance to environmental changes (pH, temperature, anions, and humic acids), presenting high removal efficiency of BSM. Radicals (IO 3 • ) and non-radicals ( 1 O 2 and electron transfer) pathways contributed to the degradation of BSM, while the latter performed a crucial role in BSM degradation. Theoretical calculations further confirmed doped of N and Mg changed the electron configuration and electrostatic potential (ESP) distribution of biochar, which was beneficial to provide more active sites for PI activation. Hydroponic experiments showed that NMg-BC/PI system could effectively degrade BSM, and its residue had no significant effect on the length and weight of soybean. The study provides a promising approach for the pollutant remediation in cold regions.
Keyphrases
  • heavy metals
  • sewage sludge
  • electron transfer
  • climate change
  • molecular dynamics simulations
  • drinking water
  • body mass index
  • weight loss
  • case report
  • weight gain
  • highly efficient
  • body weight
  • metal organic framework