Structural and dynamic inhomogeneities induced by curvature gradients in elliptic colloidal halos of paramagnetic particles.
O A Ramírez-GarzaJosé Miguel Méndez-AlcarazP González-MozuelosPublished in: The Journal of chemical physics (2018)
Paramagnetic colloidal particles distributed along an ellipse are used as a model system to study the effects of curvature gradients on the structure and dynamics of colloids in curved manifolds. Unlike what happens for circular and spherical systems, in the present case, the equilibrium one-particle distribution function displays inhomogeneities due to the changing curvature along the ellipse. The ensuing effects on the two-body correlations are also analyzed, leading to the observation of anisotropic and long-ranged effects. Another noticeable consequence is the slowing down of the self-diffusion of these particles, which for large eccentricities may induce metastable states; this is evaluated by means of the time-dependent self-distribution.