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Lasing of moiré trapped MoSe 2 /WSe 2 interlayer excitons coupled to a nanocavity.

Chenjiang QianMirco TroueJohannes FigueiredoPedro SoubeletViviana VillafañeJohannes BeierleinSebastian KlembtAndreas V StierSven HöflingAlexander W HolleitnerJonathan J Finley
Published in: Science advances (2024)
We report lasing of moiré trapped interlayer excitons (IXs) by integrating a pristine hBN-encapsulated MoSe 2 /WSe 2 heterobilayer into a high- Q (>10 4 ) nanophotonic cavity. We control the cavity-IX detuning using a magnetic field and measure their dipolar coupling strength to be 78 ± 4 micro-electron volts, fully consistent with the 82 micro-electron volts predicted by theory. The emission from the cavity mode shows clear threshold-like behavior as the transition is tuned into resonance with the cavity. We observe a superlinear power dependence accompanied by a narrowing of the linewidth as the distinct features of lasing. The onset and prominence of these threshold-like behaviors are pronounced at resonance while weak off-resonance. Our results show that a lasing transition can be induced in interacting moiré IXs with macroscopic coherence extending over the length scale of the cavity mode. Such systems raise interesting perspectives for low-power switching and synaptic nanophotonic devices using two-dimensional materials.
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