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A perovskite solar cell-photothermal-thermoelectric tandem system for enhanced solar energy utilization.

Han ZhongYangying ZhouCong WangChunlei WanKunihito KoumotoZhiping WangHong Lin
Published in: Science and technology of advanced materials (2024)
Photovoltaic-thermoelectric (PV-TE) tandem system has been considered as an effective way to fully utilize the solar spectrum, and has been demonstrated in a perovskite solar cell (PSC)-thermoelectric (TE) configuration. However, the conventional PSC-TE tandem architecture cannot convert infrared light transmitted through the upper PSC into heat effectively, impeding the heat-electricity conversion of TE devices. Herein, a semi-transparent PSC-photothermal-TE tandem system is designed for improved photothermal utilization. Through optimizing the buffer layer of the back transparent electrode, semi-transparent PSC with a power conversion efficiency (PCE) of 13% and an average transmittance of 53% in the range of 800-1500 nm was obtained. On this basis, a photothermal thin film was introduced between the semi-transparent PSC and the TE device, which increased the efficiency contribution ratio of the TE device from 14% to 19%, showing enhanced utilization of AM 1.5 G solar spectrum and improved photo-thermal-electric conversion efficiency.
Keyphrases
  • photodynamic therapy
  • cancer therapy
  • drug delivery
  • drug release
  • cell therapy
  • light emitting
  • electron transfer