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Detection of a pair density wave state in UTe 2 .

Qiangqiang GuJoseph P CarrollShuqiu WangSheng RanChristopher BroylesHasan SiddiqueeNicholas P ButchShanta R SahaJohnpierre PaglioneJ C Séamus DavisXiaolong Liu
Published in: Nature (2023)
Spin-triplet topological superconductors should exhibit many unprecedented electronic properties, including fractionalized electronic states relevant to quantum information processing. Although UTe 2 may embody such bulk topological superconductivity 1-11 , its superconductive order parameter Δ(k) remains unknown 12 . Many diverse forms for Δ(k) are physically possible 12 in such heavy fermion materials 13 . Moreover, intertwined 14,15 density waves of spin (SDW), charge (CDW) and pair (PDW) may interpose, with the latter exhibiting spatially modulating 14,15 superconductive order parameter Δ(r), electron-pair density 16-19 and pairing energy gap 17,20-23 . Hence, the newly discovered CDW state 24 in UTe 2 motivates the prospect that a PDW state may exist in this material 24,25 . To search for it, we visualize the pairing energy gap with μeV-scale energy resolution using superconductive scanning tunnelling microscopy (STM) tips 26-31 . We detect three PDWs, each with peak-to-peak gap modulations of around 10 μeV and at incommensurate wavevectors P i=1,2,3 that are indistinguishable from the wavevectors Q i=1,2,3 of the prevenient 24 CDW. Concurrent visualization of the UTe 2 superconductive PDWs and the non-superconductive CDWs shows that every P i :Q i pair exhibits a relative spatial phase δϕ ≈ π. From these observations, and given UTe 2 as a spin-triplet superconductor 12 , this PDW state should be a spin-triplet PDW 24,25 . Although such states do exist 32 in superfluid 3 He, for superconductors, they are unprecedented.
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