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Strong variation of spin-orbit torques with relative spin relaxation rates in ferrimagnets.

Lijun ZhuDaniel C Ralph
Published in: Nature communications (2023)
Spin-orbit torques (SOTs) have been widely understood as an interfacial transfer of spin that is independent of the bulk properties of the magnetic layer. Here, we report that SOTs acting on ferrimagnetic Fe x Tb 1-x layers decrease and vanish upon approaching the magnetic compensation point because the rate of spin transfer to the magnetization becomes much slower than the rate of spin relaxation into the crystal lattice due to spin-orbit scattering. These results indicate that the relative rates of competing spin relaxation processes within magnetic layers play a critical role in determining the strength of SOTs, which provides a unified understanding for the diverse and even seemingly puzzling SOT phenomena in ferromagnetic and compensated systems. Our work indicates that spin-orbit scattering within the magnet should be minimized for efficient SOT devices. We also find that the interfacial spin-mixing conductance of interfaces of ferrimagnetic alloys (such as Fe x Tb 1-x ) is as large as that of 3d ferromagnets and insensitive to the degree of magnetic compensation.
Keyphrases
  • room temperature
  • single molecule
  • density functional theory
  • transition metal
  • ionic liquid
  • molecularly imprinted
  • mass spectrometry
  • molecular dynamics simulations
  • high resolution
  • visible light