Tuning the Flat Band in Bi 2 O 2 Se by Pressure to Induce Superconductivity.
Hui TianTeng TuXilian JinChenyi LiTao LinQing DongXiaoling JingBo LiuRan LiuDa LiZhongkai LiuQuanjun LiHai-Lin PengBingbing LiuPublished in: Journal of the American Chemical Society (2024)
The discovery of superconductivity in twisted bilayer graphene has reignited enthusiasm in the field of flat-band superconductivity. However, important challenges remain, such as constructing a flat-band structure and inducing a superconducting state in materials. Here, we successfully achieved superconductivity in Bi 2 O 2 Se by pressure-tuning the flat-band electronic structure. Experimental measurements combined with theoretical calculations reveal that the occurrence of pressure-induced superconductivity at 30 GPa is associated with a flat-band electronic structure near the Fermi level. Moreover, in Bi 2 O 2 Se, a van Hove singularity is observed at the Fermi level alongside pronounced Fermi surface nesting. These remarkable features play a crucial role in promoting strong electron-phonon interactions, thus potentially enhancing the superconducting properties of the material. These findings demonstrate that pressure offers a potential experimental strategy for precisely tuning the flat band and achieving superconductivity.