Laser-Controlled Implementation of Controlled-NOT, Hadamard, SWAP, and Pauli Gates as Well as Generation of Bell States in a 3d-4f Molecular Magnet.

Using high-level ab initio many-body theory, we theoretically propose that the Dy and the Ni atoms in the [Dy 2 Ni 2 (L) 4 (NO 3 ) 2 (DMF) 2 ] real molecular magnet as well as in its core, that is, the [Dy 2 Ni 2 O 6 ] system, act as two-level qubit systems. Despite their spatial proximity we can individually control each qubit in this highly correlated real magnetic system through specially designed laser-pulse combinations. This allows us to prepare any desired two-qubit state and to build several classical and quantum logic gates, such as the two-qubit (binary) CNOT gate with three distinct laser pulses. Other quantum logic gates include the single-qubit (unary) quantum X, Y, and Z Pauli gates; the Hadamard gate (which necessitates the coherent quantum superposition of two many-body electronic states); and the SWAP gate (which plays an important role in Shor's algorithm for integer factorization). Finally, by sequentially using the achieved CNOT and Hadamard gates we are able to obtain the maximally entangled Bell states, for example, ( 1 2 )(|00⟩ + |11⟩).